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Single molecule electron transfer dynamics in complex environments

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dc.contributor.authorLeite, VBP
dc.contributor.authorAlonso, LCP
dc.contributor.authorNewton, M.
dc.contributor.authorWang, J.
dc.contributor.institutionChinese Acad Sci
dc.contributor.institutionBrookhaven Natl Lab
dc.contributor.institutionSUNY Stony Brook
dc.contributor.institutionUniversidade Estadual Paulista (Unesp)
dc.date.accessioned2014-05-20T15:26:24Z
dc.date.available2014-05-20T15:26:24Z
dc.date.issued2005-09-09
dc.description.abstractWe propose a new theoretical approach to study the kinetics of the electron transfer (ET) under the dynamical influence of the complex environments with the first passage times (FPT) of the reaction events. By measuring the mean and high order moments of FPT and their ratios, the full kinetics of ET, especially the dynamical transitions across different temperature zones, is revealed. The potential applications of the current results to single molecule electron transfer are discussed.en
dc.description.affiliationChinese Acad Sci, Changchun Inst Appl Chem, State Key Lab Electroanalyt Chem, Changchun 130022, Peoples R China
dc.description.affiliationBrookhaven Natl Lab, Dept Chem, Upton, NY 11973 USA
dc.description.affiliationSUNY Stony Brook, Dept Chem, Stony Brook, NY 11794 USA
dc.description.affiliationSUNY Stony Brook, Dept Phys, Stony Brook, NY 11794 USA
dc.format.extent4
dc.identifierhttp://dx.doi.org/10.1103/PhysRevLett.95.118301
dc.identifier.citationPhysical Review Letters. College Pk: American Physical Soc, v. 95, n. 11, 4 p., 2005.
dc.identifier.doi10.1103/PhysRevLett.95.118301
dc.identifier.fileWOS000231802000074.pdf
dc.identifier.issn0031-9007
dc.identifier.urihttp://hdl.handle.net/11449/36577
dc.identifier.wosWOS:000231802000074
dc.language.isoeng
dc.publisherAmerican Physical Soc
dc.relation.ispartofPhysical Review Letters
dc.relation.ispartofjcr8.839
dc.relation.ispartofsjr3,622
dc.rights.accessRightsAcesso aberto
dc.sourceWeb of Science
dc.titleSingle molecule electron transfer dynamics in complex environmentsen
dc.typeArtigo
dcterms.licensehttp://publish.aps.org/authors/transfer-of-copyright-agreement
dcterms.rightsHolderAmerican Physical Soc
dspace.entity.typePublication

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