Coherence characteristics of random lasing in a dye doped hybrid powder

Abstract

The photon statistics of the random laser emission of a Rhodamine B doped di-ureasil hybrid powder is investigated to evaluate its degree of coherence above threshold. Although the random laser emission is a weighted average of spatially uncorrelated radiation emitted at different positions in the sample, a spatial coherence control was achieved due to an improved detection configuration based on spatial filtering. By using this experimental approach, which also allows for fine mode discrimination and time-resolved analysis of uncoupled modes from mode competition, an area not larger than the expected coherence size of the random laser is probed. Once the spectral and temporal behavior of non-overlapping modes is characterized, an assessment of the photon-number probability distribution and the resulting second-order correlation coefficient as a function of time delay and wavelength was performed. The outcome of our single photon counting measurements revealed a high degree of temporal coherence at the time of maximum pump intensity and at wavelengths around the Rhodamine B gain maximum. (C) 2015 Elsevier B.V. All rights reserved.