Triangular-lattice anisotropic dimerized Heisenberg antiferromagnet: Stability and excitations of the quantum paramagnetic phase

Abstract

Motivated by experiments on nonmagnetic triangular-lattice Mott insulators, we study one candidate paramagnetic phase, namely the columnar dimer (or valence-bond) phase. We apply variants of the bond-operator theory to a dimerized and spatially anisotropic spin-1/2 Heisenberg model and determine its zero-temperature phase diagram and the spectrum of elementary triplet excitations (triplons). Depending on model parameters, we find that the minimum of the triplon energy is located at either a commensurate or an incommensurate wave vector. Condensation of triplons at this commensurate-incommensurate transition defines a quantum Lifshitz point, with effective dimensional reduction that possibly leads to nontrivial paramagnetic (e.g., spin-liquid) states near the closing of the triplet gap. We also discuss the two-particle decay of high-energy triplons, and we comment on the relevance of our results for the organic Mott insulator (EtMeP)-P-3[Pd(dmit)(2)](2).