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Synthesis of Main-Chain Poly(fullerene)s from a Sterically Controlled Azomethine Ylide Cycloaddition Polymerization

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dc.contributor.authorRamanitra, Hasina H.
dc.contributor.authorSantos Silva, Hugo
dc.contributor.authorBregadiolli, Bruna A. [UNESP]
dc.contributor.authorKhoukh, Abdel
dc.contributor.authorCombe, Craig M. S.
dc.contributor.authorDowland, Simon A.
dc.contributor.authorBégué, Didier
dc.contributor.authorGraeff, Carlos F. O. [UNESP]
dc.contributor.authorDagron-Lartigau, Christine
dc.contributor.authorDistler, Andreas
dc.contributor.authorMorse, Graham
dc.contributor.authorHiorns, Roger C.
dc.contributor.institutionCNRS-UMR 5254
dc.contributor.institutionUniversidade Estadual Paulista (Unesp)
dc.contributor.institutionBelectric OPV GmbH
dc.contributor.institutionUniversity Parkway
dc.date.accessioned2018-12-11T17:27:28Z
dc.date.available2018-12-11T17:27:28Z
dc.date.issued2016-03-09
dc.description.abstractFullerene is used as a monomer in this simple method to prepare soluble, well-defined polymers. The sterically controlled azomethine ylide cycloaddition polymerization of fullerene (SACAP) yields macromolecules with molecular weights of around 25 000 g mol-1. Importantly, cumbersome comonomers are employed to restrict cross-linking. Extensive characterizations, with the help of modeling studies, indicate that the polymers are regio-irregular with a majority of trans-3 isomers. Of particular interest is the exceptional ease of preparing polymers with zero metal content.en
dc.description.affiliationUniversité de Pau et des Pays de l'Adour IPREM EPCP CNRS-UMR 5254, 2 Avenue Président Angot
dc.description.affiliationUniversité de Pau et des Pays de l'Adour IPREM ECP CNRS-UMR 5254, 2 Avenue Président Angot
dc.description.affiliationDepartamento de Física-FC UNESP, Av. Luiz Edmundo Carrijo Coube, 14-01
dc.description.affiliationBelectric OPV GmbH, Landgrabenstr. 94
dc.description.affiliationMerck Chemicals Ltd. Chilworth Technical Centre University Parkway
dc.description.affiliationCNRS IPREM EPCP CNRS-UMR 5254
dc.description.affiliationUnespDepartamento de Física-FC UNESP, Av. Luiz Edmundo Carrijo Coube, 14-01
dc.description.sponsorshipFundação de Amparo à Pesquisa do Estado de São Paulo (FAPESP)
dc.description.sponsorshipCoordenação de Aperfeiçoamento de Pessoal de Nível Superior (CAPES)
dc.description.sponsorshipIdFAPESP: 2011/02205-3
dc.description.sponsorshipIdCAPES: BEX 11216-12-3
dc.format.extent1681-1691
dc.identifierhttp://dx.doi.org/10.1021/acs.macromol.5b02793
dc.identifier.citationMacromolecules, v. 49, n. 5, p. 1681-1691, 2016.
dc.identifier.doi10.1021/acs.macromol.5b02793
dc.identifier.issn1520-5835
dc.identifier.issn0024-9297
dc.identifier.scopus2-s2.0-84960341520
dc.identifier.urihttp://hdl.handle.net/11449/177863
dc.language.isoeng
dc.relation.ispartofMacromolecules
dc.relation.ispartofsjr2,419
dc.relation.ispartofsjr2,419
dc.rights.accessRightsAcesso restrito
dc.sourceScopus
dc.titleSynthesis of Main-Chain Poly(fullerene)s from a Sterically Controlled Azomethine Ylide Cycloaddition Polymerizationen
dc.typeArtigo
dspace.entity.typePublication
unesp.author.lattes5268607684223281[8]
unesp.author.orcid0000-0003-0162-8273[8]
unesp.departmentFísica - FCpt

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