Optical excitation of charge carriers from intra-bandgap states in Ce-doped SnO2 thin films

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Silva, Vitor D. L. [UNESP]
Pineiz, Tatiane F. [UNESP]
Morais, Evandro A. [UNESP]
Pinheiro, Marco A. L. [UNESP]
Scalvi, Luis Vicente de Andrade [UNESP]
Saeki, Margarida Juri [UNESP]
Rubo, Elisabete Aparecida Andrello [UNESP]

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Optical excitation of Ce3+-doped SnO2 thin films, obtained by the sol-gel-dip-coating technique, is carried out and the effects on electrical transport are evaluated. Samples are doped with O. lat% of Ce, just above the saturation limit. The excitation is done with an intensity-controlled halogen-tungsten lamp through an interference filter, yielding an excitation wavelength of 513nm, 9 nm wide (width at half intensity peak). Irradiation at low temperature (25K) yields a conductivity increase much lower than above bandgap light. Such a behavior assures the ionization of intra-bandgap defect levels, since the filter does not allow excitation of electron-hole pairs, what would happen only in the UV range (below about 350nm). The decay of intra-bandgap excited levels in the range 250-320 K is recorded, leading to a temperature dependent behavior related to a thermally excited capture cross section for the dominating defect level. © 2008 American Institute of Physics.



Cerium, Electroluminescent devices, Thin films, Tin dioxide

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AIP Conference Proceedings, v. 992, p. 1283-1288.